Abstract

The meteorological factors of the severe wintertime particulate matter (PM) air pollution problem of the city of Santiago, Chile, are investigated with newly available observations, including a 30 m tower measuring near-surface stability, winds and turbulence, as well as lower-tropospheric vertical profiles of temperature and winds measured by commercial airplanes operating from the Santiago airport (AMDAR database). Focusing on the cold season of the years 2017-2019, high-PM days are defined using an index of evening concentrations measured in the western part of the city. The diurnal cycles of the different meteorological variables computed over 25 PM episodes are compared against the overall diurnal cycles. PM episodes are associated with enhanced surface stability and weaker surface winds and turbulence during the evening and night. AMDAR vertical profiles of temperature and winds during episodes reveal a substantial lower-tropospheric warming attributed to enhanced regional subsidence, which is consistent with the shallower daytime boundary layer depth and the increased surface thermal amplitude observed during these days. An explanation for the weak surface winds during PM episodes was not evident, considering that these are clear days that would strengthen the local valley wind system. Two possible mechanisms are put forward to resolve this issue, which can be tested in the future using high-resolution numerical modeling validated with the new data described here.