Low-Temperature Photophysics of Single Nitrogen-Vacancy Centers in Diamond

Happacher, Jodok; Broadway, David A.; Bocquel, Juanita; Reiser, Patrick; Jimenéz, Alejandro; Tschudin, Märta A.; Thiel, Lucas; Rohner, Dominik; Puigibert, Marcel Li Grimau; Shields, Brendan; MAZE-RIOS, Jeronimo R.; Jacques, V.; Maletinsky, P.

Abstract

We investigate the magnetic field dependent photophysics of individual nitrogen-vacancy (NV) color centers in diamond under cryogenic conditions. At distinct magnetic fields, we observe significant reductions in the NV photoluminescence rate, which indicate a marked decrease in the optical readout efficiency of the NV???s ground state spin. We assign these dips to excited state level anticrossings, which occur at magnetic fields that strongly depend on the effective, local strain environment of the NV center. Our results offer new insights into the structure of the NVs??? excited states and a new tool for their effective characterization. Using this tool, we observe strong indications for strain-dependent variations of the NV???s orbital g factor, obtain new insights into NV charge state dynamics, and draw important conclusions regarding the applicability of NV centers for low-temperature quantum sensing.

Más información

Título según WOS: Low-Temperature Photophysics of Single Nitrogen-Vacancy Centers in Diamond
Título según SCOPUS: Low-Temperature Photophysics of Single Nitrogen-Vacancy Centers in Diamond
Título de la Revista: PHYSICAL REVIEW LETTERS
Volumen: 128
Editorial: American Physical Society
Fecha de publicación: 2022
DOI:

10.1103/PHYSREVLETT.128.177401

Notas: ISI, SCOPUS